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MestreNova is a powerful software for processing and analyzing NMR data. It can be used to determine the structure of an unknown compound by comparing its NMR spectrum to a library of known spectra. To use MestreNova for this purpose, first import the NMR spectrum of the unknown compound into the software. Then, use the "Identify" tool to search the library for spectra that match the unknown spectrum. MestreNova will then display a list of potential structures for the unknown compound. You can then use the "Analyze" tool to further refine the structure and determine the most likely candidate.